Local dynamical characteristics of a molecular aggregate under the action of the bichromatic electromagnetic field

Several dynamical characteristics of the impurity coupled to the linear molecular aggregate under the action of the bichromatic electromagnetic field are calculated. Both the exciton band and the local levels, caused by the impurity, can contribute to the local dynamical characteristics of the impurity. We have shown that the bichromatic electromagnetic field produces combined resonances, which manifest themselves in all dynamical characteristics ofthe system. We also have shown that one can observe resonance features of the dynamical characteristics at frequencies (or wavelengths) in the diapason far beyond own frequencies of the molecular aggregate and the impurity.

Key words: molecular aggregate, bichromatic electromagnetic field, local dynamical characteristics, combined resonance.

References

1. Y. V. Malykin, A. V. Sorokin, and V. P. Seminozhenko, Fiz. Nizk. Temp. 42, 551 (2016) [Low Temp. Phys. 42, 429 (2016)]. CrossRef Google Scholar

2. G. D. Scholes and G. Rumbles, Nat. Mater. 5, 683 (2006). CrossRef Google Scholar

3. S. K. Saikin, A. Eisfeld, S. Valleau, and A. Aspru-Guzik, Nanophotonics 2(1), 21 (2013). CrossRef Google Scholar

4. E. E. Jelley, Nature 138, 1009 (1936); ibid. 139, 631 (1937). CrossRef Google Scholar

5. G. Scheibe, Angew. Chemie 50, 212 (1937); ibid. 52, 631 (1939). CrossRef Google Scholar

6. F. Wurthner, T. E. Kaiser, and C. R. Saha-Muller, Angew. Chem. Int. Ed. 50, 3376 (2011). CrossRef Google Scholar

7. D. Möbius, Adv. Matter 7, 437 (1995). CrossRef Google Scholar

8. J-Aggregates, edited by W. T. Kobayashi (World Scientific Publishing, Singapore, 1996). Google Scholar

9. D. M. Eisele, J. Knoester, S. Kirstein, J. P. Rabe, and D. A. Vanden Bout, Nat. Nanotech. 4, 658 (2009). CrossRef Google Scholar

10. H. von Berlepsch and C. Böttcher, J. Phys. Chem. B 106, 3146 (2002). CrossRef Google Scholar

11. E. Lang, A. Sorokin, M. Drechsler, Y. V. Malyukin, and J. Köhler, Nano Lett. 5, 2635 (2005). CrossRef Google Scholar

12. A. S. Davydov, Theory of Molecular Excitons (Springer Science and Business Media, New York, 1971). Google Scholar

13. Excitons, edited by E. I. Rashba and M. D. Sturge (North-Holland, Amsterdam, 1982). Google Scholar

14. J. Knoester and V. M. Agranovich, in Electronic Excitations in Organic-Based Nanostructures, Thin Films and Nanostructures, edited by V. M. Agranovich and G. F. Bassani (Elsevier, Amsterdam, 2003), Vol. 31. Google Scholar

15. J. R. Lacowitz, Principles of the Fluorescent Spectroscopy (Springer, New York, 2006). Google Scholar

16. E. L. Purcell, Phys. Rev. 69, 681 (1946). CrossRef Google Scholar

17. E. I. Rashba, Opt. Spectr. 2, 568 (1957). Google Scholar

18. K. H. Drexhage, Progr. Opt. 12, 163 (1974). CrossRef Google Scholar

19. R. R. Chance, A. Prock, and R. Silbey, Adv. Chem. Phys. 37, 1 (1978). CrossRef Google Scholar

20. D. Kleppner, Phys. Rev. Lett. 47, 233 (1981). CrossRef Google Scholar

21. P. Lodahl, A. F. van Driel, I. S. Nikolaev, A. Irman, K. Overgaag, D. A. M. Vanmaekelbergh, and W. L. Vos, Nature (London) 430, 654 (2004). CrossRef Google Scholar

22. A. V. Sorokin, A. A. Zabolotskii, N. V. Pereverzev, S. L. Yefimova, Y. V. Malyukin, and A. I. Plekhanov, J. Phys. Chem. C 118, 7599 (2014). CrossRef Google Scholar

23. A. V. Sorokin, A. A. Zabolotskii, N. V. Pereverzev, I. I. Bespalova, S. L. Yefimova, Y. V. Malyukin, and A. I. Plekhanov, J. Phys. Chem. C 119, 2743 (2015). CrossRef Google Scholar

24. I. Y. Ropakova, A. V. Sorokin, A. A. Zvyagin, and Y. V. Malyukin, Fiz. Nizk. Temp. 43, 513 (2017) [Low Temp. Phys. 43, 416 (2017)]. CrossRef Google Scholar

25. A. A. Zvyagin and I. Y. Ropakova, Europhys. Lett. 117, 47005 (2017). CrossRef Google Scholar

26. A. A. Zvyagin and I. Y. Ropakova, Fiz. Nizk. Temp. 46, 805 (2020) [Low Temp. Phys. 46, 677 (2020)]. CrossRef Google Scholar

27. P. Törmä and W. L. Barnes, Rep. Progr. Phys. 78, 013901 (2015). CrossRef Google Scholar

28. P. Jordan and E. Wigner, Z. Phys. 47, 631 (1928). CrossRef Google Scholar

29. A. A. Zvyagin, Finite Size Effects in Correlated Electron Models: Exact Results (Imperial College Press, London, 2005). Google Scholar

30. A. A. Zvyagin, Phys. Rev. B 85, 134435 (2012). CrossRef Google Scholar